author_facet Zhao, Pei-Chen
Li, Wen
Huang, Wei
Li, Cheng-Hui
Zhao, Pei-Chen
Li, Wen
Huang, Wei
Li, Cheng-Hui
author Zhao, Pei-Chen
Li, Wen
Huang, Wei
Li, Cheng-Hui
spellingShingle Zhao, Pei-Chen
Li, Wen
Huang, Wei
Li, Cheng-Hui
Molecules
A Self-Healing Polymer with Fast Elastic Recovery upon Stretching
Chemistry (miscellaneous)
Analytical Chemistry
Organic Chemistry
Physical and Theoretical Chemistry
Molecular Medicine
Drug Discovery
Pharmaceutical Science
author_sort zhao, pei-chen
spelling Zhao, Pei-Chen Li, Wen Huang, Wei Li, Cheng-Hui 1420-3049 MDPI AG Chemistry (miscellaneous) Analytical Chemistry Organic Chemistry Physical and Theoretical Chemistry Molecular Medicine Drug Discovery Pharmaceutical Science http://dx.doi.org/10.3390/molecules25030597 <jats:p>The design of polymers that exhibit both good elasticity and self-healing properties is a highly challenging task. In spite of this, the literature reports highly stretchable self-healing polymers, but most of them exhibit slow elastic recovery behavior, i.e., they can only recover to their original length upon relaxation for a long time after stretching. Herein, a self-healing polymer with a fast elastic recovery property is demonstrated. We used 4-[tris(4-formylphenyl)methyl]benzaldehyde (TFPM) as a tetratopic linker to crosslink a poly(dimethylsiloxane) backbone, and obtained a self-healing polymer with high stretchability and fast elastic recovery upon stretching. The strain at break of the as-prepared polymer is observed at about 1400%. The polymer can immediately recover to its original length after being stretched. The damaged sample can be healed at room temperature with a healing efficiency up to 93% within 1 h. Such a polymer can be used for various applications, such as functioning as substrates or matrixes in soft actuators, electronic skins, biochips, and biosensors with prolonged lifetimes.</jats:p> A Self-Healing Polymer with Fast Elastic Recovery upon Stretching Molecules
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title A Self-Healing Polymer with Fast Elastic Recovery upon Stretching
title_unstemmed A Self-Healing Polymer with Fast Elastic Recovery upon Stretching
title_full A Self-Healing Polymer with Fast Elastic Recovery upon Stretching
title_fullStr A Self-Healing Polymer with Fast Elastic Recovery upon Stretching
title_full_unstemmed A Self-Healing Polymer with Fast Elastic Recovery upon Stretching
title_short A Self-Healing Polymer with Fast Elastic Recovery upon Stretching
title_sort a self-healing polymer with fast elastic recovery upon stretching
topic Chemistry (miscellaneous)
Analytical Chemistry
Organic Chemistry
Physical and Theoretical Chemistry
Molecular Medicine
Drug Discovery
Pharmaceutical Science
url http://dx.doi.org/10.3390/molecules25030597
publishDate 2020
physical 597
description <jats:p>The design of polymers that exhibit both good elasticity and self-healing properties is a highly challenging task. In spite of this, the literature reports highly stretchable self-healing polymers, but most of them exhibit slow elastic recovery behavior, i.e., they can only recover to their original length upon relaxation for a long time after stretching. Herein, a self-healing polymer with a fast elastic recovery property is demonstrated. We used 4-[tris(4-formylphenyl)methyl]benzaldehyde (TFPM) as a tetratopic linker to crosslink a poly(dimethylsiloxane) backbone, and obtained a self-healing polymer with high stretchability and fast elastic recovery upon stretching. The strain at break of the as-prepared polymer is observed at about 1400%. The polymer can immediately recover to its original length after being stretched. The damaged sample can be healed at room temperature with a healing efficiency up to 93% within 1 h. Such a polymer can be used for various applications, such as functioning as substrates or matrixes in soft actuators, electronic skins, biochips, and biosensors with prolonged lifetimes.</jats:p>
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author Zhao, Pei-Chen, Li, Wen, Huang, Wei, Li, Cheng-Hui
author_facet Zhao, Pei-Chen, Li, Wen, Huang, Wei, Li, Cheng-Hui, Zhao, Pei-Chen, Li, Wen, Huang, Wei, Li, Cheng-Hui
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description <jats:p>The design of polymers that exhibit both good elasticity and self-healing properties is a highly challenging task. In spite of this, the literature reports highly stretchable self-healing polymers, but most of them exhibit slow elastic recovery behavior, i.e., they can only recover to their original length upon relaxation for a long time after stretching. Herein, a self-healing polymer with a fast elastic recovery property is demonstrated. We used 4-[tris(4-formylphenyl)methyl]benzaldehyde (TFPM) as a tetratopic linker to crosslink a poly(dimethylsiloxane) backbone, and obtained a self-healing polymer with high stretchability and fast elastic recovery upon stretching. The strain at break of the as-prepared polymer is observed at about 1400%. The polymer can immediately recover to its original length after being stretched. The damaged sample can be healed at room temperature with a healing efficiency up to 93% within 1 h. Such a polymer can be used for various applications, such as functioning as substrates or matrixes in soft actuators, electronic skins, biochips, and biosensors with prolonged lifetimes.</jats:p>
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spelling Zhao, Pei-Chen Li, Wen Huang, Wei Li, Cheng-Hui 1420-3049 MDPI AG Chemistry (miscellaneous) Analytical Chemistry Organic Chemistry Physical and Theoretical Chemistry Molecular Medicine Drug Discovery Pharmaceutical Science http://dx.doi.org/10.3390/molecules25030597 <jats:p>The design of polymers that exhibit both good elasticity and self-healing properties is a highly challenging task. In spite of this, the literature reports highly stretchable self-healing polymers, but most of them exhibit slow elastic recovery behavior, i.e., they can only recover to their original length upon relaxation for a long time after stretching. Herein, a self-healing polymer with a fast elastic recovery property is demonstrated. We used 4-[tris(4-formylphenyl)methyl]benzaldehyde (TFPM) as a tetratopic linker to crosslink a poly(dimethylsiloxane) backbone, and obtained a self-healing polymer with high stretchability and fast elastic recovery upon stretching. The strain at break of the as-prepared polymer is observed at about 1400%. The polymer can immediately recover to its original length after being stretched. The damaged sample can be healed at room temperature with a healing efficiency up to 93% within 1 h. Such a polymer can be used for various applications, such as functioning as substrates or matrixes in soft actuators, electronic skins, biochips, and biosensors with prolonged lifetimes.</jats:p> A Self-Healing Polymer with Fast Elastic Recovery upon Stretching Molecules
spellingShingle Zhao, Pei-Chen, Li, Wen, Huang, Wei, Li, Cheng-Hui, Molecules, A Self-Healing Polymer with Fast Elastic Recovery upon Stretching, Chemistry (miscellaneous), Analytical Chemistry, Organic Chemistry, Physical and Theoretical Chemistry, Molecular Medicine, Drug Discovery, Pharmaceutical Science
title A Self-Healing Polymer with Fast Elastic Recovery upon Stretching
title_full A Self-Healing Polymer with Fast Elastic Recovery upon Stretching
title_fullStr A Self-Healing Polymer with Fast Elastic Recovery upon Stretching
title_full_unstemmed A Self-Healing Polymer with Fast Elastic Recovery upon Stretching
title_short A Self-Healing Polymer with Fast Elastic Recovery upon Stretching
title_sort a self-healing polymer with fast elastic recovery upon stretching
title_unstemmed A Self-Healing Polymer with Fast Elastic Recovery upon Stretching
topic Chemistry (miscellaneous), Analytical Chemistry, Organic Chemistry, Physical and Theoretical Chemistry, Molecular Medicine, Drug Discovery, Pharmaceutical Science
url http://dx.doi.org/10.3390/molecules25030597