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Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability
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| Zeitschriftentitel: | Membranes |
|---|---|
| Personen und Körperschaften: | , , , , |
| In: | Membranes, 9, 2019, 3, S. 35 |
| Format: | E-Article |
| Sprache: | Englisch |
| veröffentlicht: |
MDPI AG
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| Schlagwörter: |
| author_facet |
Klingberg, Patrik Wilkner, Kai Schlüter, Markus Grünauer, Judith Shishatskiy, Sergey Klingberg, Patrik Wilkner, Kai Schlüter, Markus Grünauer, Judith Shishatskiy, Sergey |
|---|---|
| author |
Klingberg, Patrik Wilkner, Kai Schlüter, Markus Grünauer, Judith Shishatskiy, Sergey |
| spellingShingle |
Klingberg, Patrik Wilkner, Kai Schlüter, Markus Grünauer, Judith Shishatskiy, Sergey Membranes Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability Filtration and Separation Chemical Engineering (miscellaneous) Process Chemistry and Technology |
| author_sort |
klingberg, patrik |
| spelling |
Klingberg, Patrik Wilkner, Kai Schlüter, Markus Grünauer, Judith Shishatskiy, Sergey 2077-0375 MDPI AG Filtration and Separation Chemical Engineering (miscellaneous) Process Chemistry and Technology http://dx.doi.org/10.3390/membranes9030035 <jats:p>The separation of carbon dioxide from coal-fired power plant flue gases using a CO2/N2-selective supported ionic liquid membrane (SILM) was investigated and the performance and stability of the membrane during operation are reported. The membrane is composed of a polyacrylonitrile (PAN) ultrafiltration membrane as a support and a selective layer of an ionic liquid (IL), 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide (EMIM Tf2N). The feasibility of large-scale SILM production was demonstrated by the formation of a square-meter-scale membrane and preparation of a membrane module. A flat-sheet envelope-type SILM module containing 0.67 m2 of the membrane was assembled. Prior to real flue gas operation, the separation behaviour of the membrane was investigated with single gases. The stability of the SILM during the test stand and pilot plant operation using real power plant flue gases is reported. The volume fraction of carbon dioxide in the flue gas was raised from approx. 14 vol. % (feed) to 40 vol. % (permeate). However, issues concerning the membrane stability were found when SO3 aerosols in large quantities were present in the flue gas.</jats:p> Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability Membranes |
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| title |
Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability |
| title_unstemmed |
Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability |
| title_full |
Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability |
| title_fullStr |
Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability |
| title_full_unstemmed |
Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability |
| title_short |
Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability |
| title_sort |
separation of carbon dioxide from real power plant flue gases by gas permeation using a supported ionic liquid membrane: an investigation of membrane stability |
| topic |
Filtration and Separation Chemical Engineering (miscellaneous) Process Chemistry and Technology |
| url |
http://dx.doi.org/10.3390/membranes9030035 |
| publishDate |
2019 |
| physical |
35 |
| description |
<jats:p>The separation of carbon dioxide from coal-fired power plant flue gases using a CO2/N2-selective supported ionic liquid membrane (SILM) was investigated and the performance and stability of the membrane during operation are reported. The membrane is composed of a polyacrylonitrile (PAN) ultrafiltration membrane as a support and a selective layer of an ionic liquid (IL), 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide (EMIM Tf2N). The feasibility of large-scale SILM production was demonstrated by the formation of a square-meter-scale membrane and preparation of a membrane module. A flat-sheet envelope-type SILM module containing 0.67 m2 of the membrane was assembled. Prior to real flue gas operation, the separation behaviour of the membrane was investigated with single gases. The stability of the SILM during the test stand and pilot plant operation using real power plant flue gases is reported. The volume fraction of carbon dioxide in the flue gas was raised from approx. 14 vol. % (feed) to 40 vol. % (permeate). However, issues concerning the membrane stability were found when SO3 aerosols in large quantities were present in the flue gas.</jats:p> |
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| author | Klingberg, Patrik, Wilkner, Kai, Schlüter, Markus, Grünauer, Judith, Shishatskiy, Sergey |
| author_facet | Klingberg, Patrik, Wilkner, Kai, Schlüter, Markus, Grünauer, Judith, Shishatskiy, Sergey, Klingberg, Patrik, Wilkner, Kai, Schlüter, Markus, Grünauer, Judith, Shishatskiy, Sergey |
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| description | <jats:p>The separation of carbon dioxide from coal-fired power plant flue gases using a CO2/N2-selective supported ionic liquid membrane (SILM) was investigated and the performance and stability of the membrane during operation are reported. The membrane is composed of a polyacrylonitrile (PAN) ultrafiltration membrane as a support and a selective layer of an ionic liquid (IL), 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide (EMIM Tf2N). The feasibility of large-scale SILM production was demonstrated by the formation of a square-meter-scale membrane and preparation of a membrane module. A flat-sheet envelope-type SILM module containing 0.67 m2 of the membrane was assembled. Prior to real flue gas operation, the separation behaviour of the membrane was investigated with single gases. The stability of the SILM during the test stand and pilot plant operation using real power plant flue gases is reported. The volume fraction of carbon dioxide in the flue gas was raised from approx. 14 vol. % (feed) to 40 vol. % (permeate). However, issues concerning the membrane stability were found when SO3 aerosols in large quantities were present in the flue gas.</jats:p> |
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| institution | DE-D275, DE-Bn3, DE-Brt1, DE-Zwi2, DE-D161, DE-Gla1, DE-Zi4, DE-15, DE-Pl11, DE-Rs1, DE-105, DE-14, DE-Ch1, DE-L229 |
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| mega_collection | MDPI AG (CrossRef) |
| physical | 35 |
| publishDate | 2019 |
| publishDateSort | 2019 |
| publisher | MDPI AG |
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| series | Membranes |
| source_id | 49 |
| spelling | Klingberg, Patrik Wilkner, Kai Schlüter, Markus Grünauer, Judith Shishatskiy, Sergey 2077-0375 MDPI AG Filtration and Separation Chemical Engineering (miscellaneous) Process Chemistry and Technology http://dx.doi.org/10.3390/membranes9030035 <jats:p>The separation of carbon dioxide from coal-fired power plant flue gases using a CO2/N2-selective supported ionic liquid membrane (SILM) was investigated and the performance and stability of the membrane during operation are reported. The membrane is composed of a polyacrylonitrile (PAN) ultrafiltration membrane as a support and a selective layer of an ionic liquid (IL), 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide (EMIM Tf2N). The feasibility of large-scale SILM production was demonstrated by the formation of a square-meter-scale membrane and preparation of a membrane module. A flat-sheet envelope-type SILM module containing 0.67 m2 of the membrane was assembled. Prior to real flue gas operation, the separation behaviour of the membrane was investigated with single gases. The stability of the SILM during the test stand and pilot plant operation using real power plant flue gases is reported. The volume fraction of carbon dioxide in the flue gas was raised from approx. 14 vol. % (feed) to 40 vol. % (permeate). However, issues concerning the membrane stability were found when SO3 aerosols in large quantities were present in the flue gas.</jats:p> Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability Membranes |
| spellingShingle | Klingberg, Patrik, Wilkner, Kai, Schlüter, Markus, Grünauer, Judith, Shishatskiy, Sergey, Membranes, Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability, Filtration and Separation, Chemical Engineering (miscellaneous), Process Chemistry and Technology |
| title | Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability |
| title_full | Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability |
| title_fullStr | Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability |
| title_full_unstemmed | Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability |
| title_short | Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability |
| title_sort | separation of carbon dioxide from real power plant flue gases by gas permeation using a supported ionic liquid membrane: an investigation of membrane stability |
| title_unstemmed | Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability |
| topic | Filtration and Separation, Chemical Engineering (miscellaneous), Process Chemistry and Technology |
| url | http://dx.doi.org/10.3390/membranes9030035 |