SOLR
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1797818056398864384 |
| author |
Zhang, Jian |
| author2 |
Wang, Tao, Pohl, Darius, Rellinghaus, Bernd, Dong, Renhao, Liu, Shaohua, Zhuang, Xiaodong, Feng, Xinliang |
| author2_role |
, , , , , , |
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t w tw, d p dp, b r br, r d rd, s l sl, x z xz, x f xf |
| author_facet |
Zhang, Jian, Wang, Tao, Pohl, Darius, Rellinghaus, Bernd, Dong, Renhao, Liu, Shaohua, Zhuang, Xiaodong, Feng, Xinliang |
| author_role |
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| author_sort |
Zhang, Jian |
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Library A |
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sid-22-col-qucosa |
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Angewandte Chemie: a journal of the Gesellschaft Deutscher Chemiker International Edition (2016), 55(23). S. 6702-6707. ISSN: 1521-3773. DOI: 10.1002/anie.201602237 |
| contents |
To achieve sustainable production of H2 fuel through water splitting, low-cost electrocatalysts for hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) are required to replace Pt and IrO2 catalysts. Here, for the first time, we present the interface engineering of novel MoS2/Ni3S2 heterostructures, in which abundant interfaces are formed. For OER, such MoS2/Ni3S2 heterostructures show an extremely low overpotential of ~218 mV at 10 mA cm-2, which is superior to that of the state-of-the-art OER electrocatalysts. Using MoS2/Ni3S2 heterostructures as bifunctional electrocatalysts, an alkali electrolyser delivers a current density of 10 mA cm-2 at a very low cell voltage of ~1.56 V. In combination with density function theory (DFT) calculations, this study demonstrates that the constructed interfaces synergistically favor the chemisorption of hydrogen and oxygencontaining intermediates, thus accelerating the overall electrochemical water splitting. |
| dewey-full |
540 |
| dewey-hundreds |
500 - Natural sciences and mathematics |
| dewey-ones |
540 - Chemistry and allied sciences |
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540 |
| dewey-search |
540 |
| dewey-sort |
3540 |
| dewey-tens |
540 - Chemistry and allied sciences |
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Online, Free |
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Chemie und Pharmazie |
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science-chemistry |
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Article, E-Article |
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text-online-journal-child |
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Journal |
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Article, E-Article |
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ElectronicArticle |
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Article, E-Article |
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Article, E-Article |
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E-Article |
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not assigned |
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Angewandte Chemie: a journal of the Gesellschaft Deutscher Chemiker International Edition (2016), 55(23). S. 6702-6707. ISSN: 1521-3773. DOI: 10.1002/anie.201602237 |
| id |
22-14-qucosa-235457 |
| illustrated |
Not Illustrated |
| imprint |
Weinheim, Wiley-VCH Verlag |
| imprint_str_mv |
Online-Ausg.: 2018 |
| institution |
DE-105, DE-Gla1, DE-Brt1, DE-D161, DE-540, DE-Pl11, DE-Rs1, DE-Bn3, DE-Zi4, DE-Zwi2, DE-D117, DE-Mh31, DE-D275, DE-Ch1, DE-15, DE-D13, DE-L242, DE-L229, DE-L328 |
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English |
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2024-05-01T03:08:24.916Z |
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zhang2018interfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivityinterfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivity |
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Qucosa |
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2018 |
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Weinheim |
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Wiley-VCH Verlag |
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14-qucosa-235457 |
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Zhang, Jian, Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity, Weinheim Wiley-VCH Verlag, Online-Ausg. 2018 Online-Ressource (Text) Saechsische Landesbibliothek- Staats- und Universitaetsbibliothek Dresden, To achieve sustainable production of H2 fuel through water splitting, low-cost electrocatalysts for hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) are required to replace Pt and IrO2 catalysts. Here, for the first time, we present the interface engineering of novel MoS2/Ni3S2 heterostructures, in which abundant interfaces are formed. For OER, such MoS2/Ni3S2 heterostructures show an extremely low overpotential of ~218 mV at 10 mA cm-2, which is superior to that of the state-of-the-art OER electrocatalysts. Using MoS2/Ni3S2 heterostructures as bifunctional electrocatalysts, an alkali electrolyser delivers a current density of 10 mA cm-2 at a very low cell voltage of ~1.56 V. In combination with density function theory (DFT) calculations, this study demonstrates that the constructed interfaces synergistically favor the chemisorption of hydrogen and oxygencontaining intermediates, thus accelerating the overall electrochemical water splitting., Grenzflächentechnik, Wasserspaltung, Elektrokatalysatoren, Nickelsulfid, Molybdändisulfid, Interface Engineering, Water Splitting, Electrocatalysts, Nickel Sulfide, Molybdenum Disulfide, Wang, Tao, Pohl, Darius, Rellinghaus, Bernd, Dong, Renhao, Liu, Shaohua, Zhuang, Xiaodong, Feng, Xinliang, Angewandte Chemie: a journal of the Gesellschaft Deutscher Chemiker International Edition (2016), 55(23). S. 6702-6707. ISSN: 1521-3773. DOI: 10.1002/anie.201602237, text/html https://nbn-resolving.org/urn:nbn:de:bsz:14-qucosa-235457 Online-Zugriff |
| spellingShingle |
Zhang, Jian, Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity: Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity, To achieve sustainable production of H2 fuel through water splitting, low-cost electrocatalysts for hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) are required to replace Pt and IrO2 catalysts. Here, for the first time, we present the interface engineering of novel MoS2/Ni3S2 heterostructures, in which abundant interfaces are formed. For OER, such MoS2/Ni3S2 heterostructures show an extremely low overpotential of ~218 mV at 10 mA cm-2, which is superior to that of the state-of-the-art OER electrocatalysts. Using MoS2/Ni3S2 heterostructures as bifunctional electrocatalysts, an alkali electrolyser delivers a current density of 10 mA cm-2 at a very low cell voltage of ~1.56 V. In combination with density function theory (DFT) calculations, this study demonstrates that the constructed interfaces synergistically favor the chemisorption of hydrogen and oxygencontaining intermediates, thus accelerating the overall electrochemical water splitting., Grenzflächentechnik, Wasserspaltung, Elektrokatalysatoren, Nickelsulfid, Molybdändisulfid, Interface Engineering, Water Splitting, Electrocatalysts, Nickel Sulfide, Molybdenum Disulfide |
| title |
Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity: Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity |
| title_auth |
Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity |
| title_full |
Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity |
| title_fullStr |
Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity |
| title_full_unstemmed |
Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity |
| title_in_hierarchy |
|
| title_short |
Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity |
| title_sort |
interface engineering of mos2/ni3s2 heterostructures for highly enhanced electrochemical overall water splitting activity interface engineering of mos2/ni3s2 heterostructures for highly enhanced electrochemical overall water splitting activity |
| title_sub |
Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity |
| title_unstemmed |
Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity: Interface Engineering of MoS2/Ni3S2 Heterostructures for Highly Enhanced Electrochemical Overall Water Splitting Activity |
| topic |
Grenzflächentechnik, Wasserspaltung, Elektrokatalysatoren, Nickelsulfid, Molybdändisulfid, Interface Engineering, Water Splitting, Electrocatalysts, Nickel Sulfide, Molybdenum Disulfide |
| topic_facet |
Grenzflächentechnik, Wasserspaltung, Elektrokatalysatoren, Nickelsulfid, Molybdändisulfid, Interface Engineering, Water Splitting, Electrocatalysts, Nickel Sulfide, Molybdenum Disulfide |
| url |
https://nbn-resolving.org/urn:nbn:de:bsz:14-qucosa-235457 |
| urn |
urn:nbn:de:bsz:14-qucosa-235457 |
| work_keys_str_mv |
AT zhangjian interfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivityinterfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivity, AT wangtao interfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivityinterfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivity, AT pohldarius interfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivityinterfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivity, AT rellinghausbernd interfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivityinterfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivity, AT dongrenhao interfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivityinterfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivity, AT liushaohua interfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivityinterfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivity, AT zhuangxiaodong interfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivityinterfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivity, AT fengxinliang interfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivityinterfaceengineeringofmos2ni3s2heterostructuresforhighlyenhancedelectrochemicaloverallwatersplittingactivity |
