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Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability
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Zeitschriftentitel: | Advanced Functional Materials |
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Personen und Körperschaften: | , , , , |
In: | Advanced Functional Materials, 26, 2016, 27, S. 4896-4905 |
Format: | E-Article |
Sprache: | Englisch |
veröffentlicht: |
Wiley
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Schlagwörter: |
author_facet |
Lee, Seung Goo Lee, Hyundo Gupta, Ankur Chang, Sehoon Doyle, Patrick S. Lee, Seung Goo Lee, Hyundo Gupta, Ankur Chang, Sehoon Doyle, Patrick S. |
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author |
Lee, Seung Goo Lee, Hyundo Gupta, Ankur Chang, Sehoon Doyle, Patrick S. |
spellingShingle |
Lee, Seung Goo Lee, Hyundo Gupta, Ankur Chang, Sehoon Doyle, Patrick S. Advanced Functional Materials Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability Electrochemistry Condensed Matter Physics Biomaterials Electronic, Optical and Magnetic Materials |
author_sort |
lee, seung goo |
spelling |
Lee, Seung Goo Lee, Hyundo Gupta, Ankur Chang, Sehoon Doyle, Patrick S. 1616-301X 1616-3028 Wiley Electrochemistry Condensed Matter Physics Biomaterials Electronic, Optical and Magnetic Materials http://dx.doi.org/10.1002/adfm.201600573 <jats:p>Micromodels with simplified porous microfluidic systems are widely used to mimic the underground oil‐reservoir environment for multiphase flow studies, enhanced oil recovery, and reservoir network mapping. However, previous micromodels cannot replicate the length scales and geochemistry of carbonate because of their material limitations. Here a simple method is introduced to create calcium carbonate (CaCO<jats:sub>3</jats:sub>) micromodels composed of in situ grown CaCO<jats:sub>3</jats:sub>. CaCO<jats:sub>3</jats:sub> nanoparticles/polymer composite microstructures are built in microfluidic channels by photopatterning, and CaCO<jats:sub>3</jats:sub> nanoparticles are selectively grown in situ from these microstructures by supplying Ca<jats:sup>2+</jats:sup>, CO<jats:sub>3</jats:sub><jats:sup>2−</jats:sup> ions rich, supersaturated solutions. This approach enables us to fabricate synthetic CaCO<jats:sub>3</jats:sub> reservoir micromodels having dynamically tunable geometries with submicrometer pore‐length scales and controlled wettability. Using this new method, acid fracturing and an immiscible fluid displacement process are demonstrated used in real oil field applications to visualize pore‐scale fluid–carbonate interactions in real time.</jats:p> Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability Advanced Functional Materials |
doi_str_mv |
10.1002/adfm.201600573 |
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Online |
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Technik Physik Chemie und Pharmazie Biologie |
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Advanced Functional Materials |
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title |
Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability |
title_unstemmed |
Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability |
title_full |
Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability |
title_fullStr |
Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability |
title_full_unstemmed |
Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability |
title_short |
Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability |
title_sort |
site‐selective in situ grown calcium carbonate micromodels with tunable geometry, porosity, and wettability |
topic |
Electrochemistry Condensed Matter Physics Biomaterials Electronic, Optical and Magnetic Materials |
url |
http://dx.doi.org/10.1002/adfm.201600573 |
publishDate |
2016 |
physical |
4896-4905 |
description |
<jats:p>Micromodels with simplified porous microfluidic systems are widely used to mimic the underground oil‐reservoir environment for multiphase flow studies, enhanced oil recovery, and reservoir network mapping. However, previous micromodels cannot replicate the length scales and geochemistry of carbonate because of their material limitations. Here a simple method is introduced to create calcium carbonate (CaCO<jats:sub>3</jats:sub>) micromodels composed of in situ grown CaCO<jats:sub>3</jats:sub>. CaCO<jats:sub>3</jats:sub> nanoparticles/polymer composite microstructures are built in microfluidic channels by photopatterning, and CaCO<jats:sub>3</jats:sub> nanoparticles are selectively grown in situ from these microstructures by supplying Ca<jats:sup>2+</jats:sup>, CO<jats:sub>3</jats:sub><jats:sup>2−</jats:sup> ions rich, supersaturated solutions. This approach enables us to fabricate synthetic CaCO<jats:sub>3</jats:sub> reservoir micromodels having dynamically tunable geometries with submicrometer pore‐length scales and controlled wettability. Using this new method, acid fracturing and an immiscible fluid displacement process are demonstrated used in real oil field applications to visualize pore‐scale fluid–carbonate interactions in real time.</jats:p> |
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author | Lee, Seung Goo, Lee, Hyundo, Gupta, Ankur, Chang, Sehoon, Doyle, Patrick S. |
author_facet | Lee, Seung Goo, Lee, Hyundo, Gupta, Ankur, Chang, Sehoon, Doyle, Patrick S., Lee, Seung Goo, Lee, Hyundo, Gupta, Ankur, Chang, Sehoon, Doyle, Patrick S. |
author_sort | lee, seung goo |
container_issue | 27 |
container_start_page | 4896 |
container_title | Advanced Functional Materials |
container_volume | 26 |
description | <jats:p>Micromodels with simplified porous microfluidic systems are widely used to mimic the underground oil‐reservoir environment for multiphase flow studies, enhanced oil recovery, and reservoir network mapping. However, previous micromodels cannot replicate the length scales and geochemistry of carbonate because of their material limitations. Here a simple method is introduced to create calcium carbonate (CaCO<jats:sub>3</jats:sub>) micromodels composed of in situ grown CaCO<jats:sub>3</jats:sub>. CaCO<jats:sub>3</jats:sub> nanoparticles/polymer composite microstructures are built in microfluidic channels by photopatterning, and CaCO<jats:sub>3</jats:sub> nanoparticles are selectively grown in situ from these microstructures by supplying Ca<jats:sup>2+</jats:sup>, CO<jats:sub>3</jats:sub><jats:sup>2−</jats:sup> ions rich, supersaturated solutions. This approach enables us to fabricate synthetic CaCO<jats:sub>3</jats:sub> reservoir micromodels having dynamically tunable geometries with submicrometer pore‐length scales and controlled wettability. Using this new method, acid fracturing and an immiscible fluid displacement process are demonstrated used in real oil field applications to visualize pore‐scale fluid–carbonate interactions in real time.</jats:p> |
doi_str_mv | 10.1002/adfm.201600573 |
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series | Advanced Functional Materials |
source_id | 49 |
spelling | Lee, Seung Goo Lee, Hyundo Gupta, Ankur Chang, Sehoon Doyle, Patrick S. 1616-301X 1616-3028 Wiley Electrochemistry Condensed Matter Physics Biomaterials Electronic, Optical and Magnetic Materials http://dx.doi.org/10.1002/adfm.201600573 <jats:p>Micromodels with simplified porous microfluidic systems are widely used to mimic the underground oil‐reservoir environment for multiphase flow studies, enhanced oil recovery, and reservoir network mapping. However, previous micromodels cannot replicate the length scales and geochemistry of carbonate because of their material limitations. Here a simple method is introduced to create calcium carbonate (CaCO<jats:sub>3</jats:sub>) micromodels composed of in situ grown CaCO<jats:sub>3</jats:sub>. CaCO<jats:sub>3</jats:sub> nanoparticles/polymer composite microstructures are built in microfluidic channels by photopatterning, and CaCO<jats:sub>3</jats:sub> nanoparticles are selectively grown in situ from these microstructures by supplying Ca<jats:sup>2+</jats:sup>, CO<jats:sub>3</jats:sub><jats:sup>2−</jats:sup> ions rich, supersaturated solutions. This approach enables us to fabricate synthetic CaCO<jats:sub>3</jats:sub> reservoir micromodels having dynamically tunable geometries with submicrometer pore‐length scales and controlled wettability. Using this new method, acid fracturing and an immiscible fluid displacement process are demonstrated used in real oil field applications to visualize pore‐scale fluid–carbonate interactions in real time.</jats:p> Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability Advanced Functional Materials |
spellingShingle | Lee, Seung Goo, Lee, Hyundo, Gupta, Ankur, Chang, Sehoon, Doyle, Patrick S., Advanced Functional Materials, Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability, Electrochemistry, Condensed Matter Physics, Biomaterials, Electronic, Optical and Magnetic Materials |
title | Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability |
title_full | Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability |
title_fullStr | Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability |
title_full_unstemmed | Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability |
title_short | Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability |
title_sort | site‐selective in situ grown calcium carbonate micromodels with tunable geometry, porosity, and wettability |
title_unstemmed | Site‐Selective In Situ Grown Calcium Carbonate Micromodels with Tunable Geometry, Porosity, and Wettability |
topic | Electrochemistry, Condensed Matter Physics, Biomaterials, Electronic, Optical and Magnetic Materials |
url | http://dx.doi.org/10.1002/adfm.201600573 |